Structure-Function Relationships in Temperature Effects on Bacterial Luciferases: Nothing Is Perfect

Описание

Тип публикации: статья из журнала

Год издания: 2022

Идентификатор DOI: 10.3390/ijms23158119

Ключевые слова: bacterial luciferase, differential scanning calorimetry, enzyme activity, molecular dynamics, protein stability, sucrose, thermal denaturation, thermal inactivationalkanal monooxygenase (fmn linked), 9014-00-0, sucrose, 122880-25-5, 57-50-1, luciferases, luciferases, bacterial

Аннотация: The evaluation of temperature effects on the structure and function of enzymes is necessary to understand the mechanisms underlying their adaptation to a constantly changing environment. In the current study, we investigated the influence of temperature variation on the activity, structural dynamics, thermal inactivation and denatuПоказать полностьюration of Photobacterium leiognathi and Vibrio harveyi luciferases belonging to different subfamilies, as well as the role of sucrose in maintaining the enzymes functioning and stability. We used the stopped-flow technique, differential scanning calorimetry and molecular dynamics to study the activity, inactivation rate, denaturation and structural features of the enzymes under various temperatures. It was found that P. leiognathi luciferase resembles the properties of cold-adapted enzymes with high activity in a narrow temperature range and slightly lower thermal stability than V. harveyi luciferase, which is less active, but more thermostable. Differences in activity at the studied temperatures can be associated with the peculiarities of the mobile loop conformational changes. The presence of sucrose does not provide an advantage in activity but increases the stability of the enzymes. Differential scanning calorimetry experiments showed that luciferases probably follow different denaturation schemes.

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Издание

Журнал: International journal of molecular sciences

Выпуск журнала: Vol. 23, Is. 15

ISSN журнала: 14220067

Издатель: NLM (Medline)

Персоны

  • Deeva A.A. (Biophysics Department, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation)
  • Lisitsa A.E. (Biophysics Department, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation)
  • Sukovatyi L.A. (Biophysics Department, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation)
  • Melnik T.N. (Institute of Protein Research, Russian Academy of Sciences, Pushchino, 142290, Russian Federation)
  • Kratasyuk V.A. (Biophysics Department, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation, Institute of Biophysics, Siberian Branch of Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation)
  • Nemtseva E.V. (Biophysics Department, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation, Institute of Biophysics, Siberian Branch of Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation)

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