Тип публикации: статья из журнала

Год издания: 2024

Идентификатор DOI: 10.1002/lpor.202400468

Аннотация: <jats:title>Abstract</jats:title><jats:p>Upconversion (UC) process involves diverse energy levels and photoluminescence modes, however, it faces the challenge of concentration quenching of the doped lanthanide ions with multiple luminescence centers. Herein, Yb<jats:sup>3+</jats:sup>/Ho<jats:sup>3+</jats:sup> and Yb<jats:sup>3+</jaПоказать полностьюts:sup>/Tm<jats:sup>3+</jats:sup> are heavily codoped into the lead-free halide double perovskite single crystal Cs<jats:sub>2</jats:sub>NaErCl<jats:sub>6</jats:sub>, enabling the controlled energy transfer UC process, and accordingly, the UC materials exhibit anti-concentration-quenching owing to the defect tolerance characters. Depending on different doping couples, the UC materials show green and red emissions under the 980 nm laser excitations. Moreover, the green-to-red emission ratio in Yb<jats:sup>3+</jats:sup>/Tm<jats:sup>3+</jats:sup> codoped Cs<jats:sub>2</jats:sub>NaErCl<jats:sub>6</jats:sub> changes dynamically with the increasing pumping intensity due to the different sensitivities of the excited energy levels. This study provides a renewed direction of the lanthanide ions heavily-doped halide double perovskites toward UC materials and facilitates the development of new smart luminescence materials for optical information storage applications.</jats:p>

Журнал: Laser &amp; Photonics Reviews

ISSN журнала: 18638880

Издатель: Wiley - VCH Verlag GmbH &amp; CO. KGaA

• Tang Baoling (Key Laboratory for Biobased Materials and Energy of Ministry of Education, College of Materials and Energy South China Agricultural University Guangzhou 510642 China)
• Zhou Xinquan (State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques School of Physics and Optoelectronics South China University of Technology Guangzhou 510641 China)
• Li Tianrui (Key Laboratory for Biobased Materials and Energy of Ministry of Education, College of Materials and Energy South China Agricultural University Guangzhou 510642 China)
• Li Liang (State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques School of Physics and Optoelectronics South China University of Technology Guangzhou 510641 China)
• Zhang Haoran (Key Laboratory for Biobased Materials and Energy of Ministry of Education, College of Materials and Energy South China Agricultural University Guangzhou 510642 China)
• Molokeev Maxim (Institute of Engineering Physics and Radioelectronic of Siberian Federal University Krasnoyarsk 660041 Russia)
• Golovnev Nicolay (Institute of Engineering Physics and Radioelectronic of Siberian Federal University Krasnoyarsk 660041 Russia)
• Xia Zhiguo (State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques School of Physics and Optoelectronics South China University of Technology Guangzhou 510641 China)
• Lei Bingfu (Key Laboratory for Biobased Materials and Energy of Ministry of Education, College of Materials and Energy South China Agricultural University Guangzhou 510642 China)

• Ядро РИНЦ (eLIBRARY.RU)