Phase separation in the Bi2O3-SiO2 system. Effect of cooling conditions on the phase composition and microstructure of solidification products

Описание

Тип публикации: статья из журнала

Год издания: 2021

Идентификатор DOI: 10.1007/s11172-021-3240-1

Ключевые слова: bismuth silicate, glass transition, macroscopic phase separation in the melt, melt crystallization, melt heat treatment, metastable phase

Аннотация: The effect of heat treatment conditions (temperature and time of isothermal holding, temperature of the start of cooling and cooling conditions) of a melt containing 50 mol.% Bi2O3 and 50 mol.% SiO2 on the phase composition and macro- and microstructure of solidification products was studied. The temperatures and ranges of macroscoПоказать полностьюpic phase separation of the melt were determined. Using physicochemical methods (powder X-ray diffraction, optical and scanning electron microscopy, and atomic absorption analysis), it was established that depending on the melt cooling conditions, solidification gives crystals of metastable bismuth silicate Bi2SiO5, or a mixture of crystalline phases and glass, or glass. The crucial influence of the holding temperature and time and the melt cooling rate on the crystallization of metastable Bi2SiO5 and formation of crystals of stable phases was demonstrated. © 2021, Springer Science+Business Media LLC.

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Издание

Журнал: Russian Chemical Bulletin

Выпуск журнала: Vol. 70, Is. 8

Номера страниц: 1462-1470

ISSN журнала: 10665285

Издатель: Springer

Персоны

  • Bermeshev T.V. (Siberian Fed Univ, 79 Prosp Svobodny, Krasnoyarsk 660041, Russia)
  • Zhereb V.P. (Siberian Fed Univ, 79 Prosp Svobodny, Krasnoyarsk 660041, Russia; MF Reshetnev Siberian State Univ Sci & Technol, 31 Prosp Im Gazety Krasnoyarsky Rabochy, Krasnoyarsk 660037, Russia)
  • Tas-Ool R.N. (Siberian Fed Univ, 79 Prosp Svobodny, Krasnoyarsk 660041, Russia)
  • Mazurova E.V. (Russian Acad Sci, Siberian Branch, Inst Chem & Chem Technol, Build 24,50 Akademgorodok, Krasnoyarsk 660036, Russia)
  • Metelitsa S.I. (Siberian Fed Univ, Sci Engn Res Ctr Kristall, 79 Prosp Svobodny, Krasnoyarsk 660041, Russia)

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