Тип публикации: статья из журнала
Год издания: 2018
Идентификатор DOI: 10.17516/1997-1397-2018-11-2-159-170
Ключевые слова: superexchange, optically excited states, Mott-Hubbard insulator
Аннотация: We investigated the effects of excited many-electron states in the optical control of the magnetic state in undoped Mott-Hubbard insulator. To derive the spin Hamiltonian in material under optical pumping we have used many-electron approach based on the X-operator representation. Extending the projection operators approach on arbitПоказать полностьюrary energy spectra of the Mott-Hubbard insulator, we obtained the Hamiltonian of superexchange interaction in analytical form. The Hamiltonian includes the spin-excitor variables which are usually missing in discussion on the magnetic response to optical pumping, and is not additive over contributions from the ground and optically excited states. As a test, a microscopic background for the optical induced superexchange was analyzed in La2CuO4 (further La214).
Журнал: JOURNAL OF SIBERIAN FEDERAL UNIVERSITY-MATHEMATICS & PHYSICS
Выпуск журнала: Vol. 11, Is. 2
Номера страниц: 159-170
ISSN журнала: 19971397
Место издания: KRASNOYARSK
Издатель: SIBERIAN FEDERAL UNIV