Effect of mechanical activation on the thermoelectric properties of Sr1-xSmxTiO3 ceramics : научное издание

Описание

Тип публикации: статья из журнала

Год издания: 2021

Идентификатор DOI: 10.1016/j.ceramint.2021.07.060

Ключевые слова: strontium titanate solid solutions, thermoelectric oxide materials, mechanochemical activation

Аннотация: The Sr1-xSmxTiO3 (x = 0.025, 0.05, 0.075, 0.1, 0.2) strontium titanate solid solutions were prepared from oxides and carbonates using a conventional ceramic technology based on the mechanochemical activation. The electrical conductivity and Seebeck coefficient of the synthesized compounds were measured in the temperature range fromПоказать полностью300 to 800 K. We found that the properties of the samples significantly depend on the preliminary mechanochemical activation. The thermoelectric power factor attains maximum value in the hydrogen reduced samples with concentration of x = 0.05 and 0.075 obtained from nanoparticles: 5.5 mu W/(cm.K-2) for Sr0.95Sm0.05TiO3 (580 K) and 4.10 mu W/(cm.K-2) for Sr0.925Sm0.075TiO3 (650 K). An increase in the annealing temperature of mechanically activated samples leads to an even greater increase in electrical conductivity and power factor: 9.2 mu W/(cm.K-2) for Sr0.925Sm0.075TiO3 (650 K).

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Издание

Журнал: CERAMICS INTERNATIONAL

Выпуск журнала: Vol. 47, Is. 20

Номера страниц: 28992-28999

ISSN журнала: 02728842

Место издания: OXFORD

Издатель: ELSEVIER SCI LTD

Персоны

  • Orlov Yu S. (Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Krasnoyarsk 660036, Russia; Siberian Fed Univ, Krasnoyarsk 660041, Russia)
  • Vereshchagin S.N. (Russian Acad Sci, Inst Chem & Chem Technol, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia)
  • Novikov S.V (Ioffe Inst, St Petersburg 194021, Russia)
  • Burkov A.T. (Ioffe Inst, St Petersburg 194021, Russia)
  • Borus A.A. (Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Krasnoyarsk 660036, Russia)
  • Sitnikov M.V (Siberian Fed Univ, Krasnoyarsk 660041, Russia)
  • Solovyov L.A. (Russian Acad Sci, Inst Chem & Chem Technol, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia)
  • Volochaev M.N. (Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Krasnoyarsk 660036, Russia)
  • Dudnikov V.A. (Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Krasnoyarsk 660036, Russia; Siberian Fed Univ, Krasnoyarsk 660041, Russia)

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